Herbert family, Earls of Powis (addnl): corresp, deeds and documents 1580-1868
Lloyd George family (addnl): papers incl letters to David Lloyd George and papers of Gwilym Lloyd George (NLW MSS unnumbered)
Robert Jones Derfel (1824-1905), writer and radical: corresp and papers (NLW MSS 23440-62)
Dr Thomas Iorwerth Ellis (1899-1970), educationist: corresp and papers
Augustus Edwin John (1878-1961), painter and etcher, and Gwen John (1876-1939), painter (addnl): papers (NLW MSS 23508-10)
Glyn Jones (1905-95), poet. short-story writer and novelist (addnl): corresp, literary, family and personal papers (NLW MSS unnumbered)
Gwyn Jones (b1907), scholar, novelist and short-story writer (addnl): corresp and literary papers
Ieuan Wyn Jones, Plaid Cymru MP: constituency corresp and papers 1987-95
William Ronald Rhys Jones (1915-87), editor and poet as Keidrych Rhys (addnl): corresp, literary and personal papers (NLW MSS 23416-29)
Lady Amy Parry-Williams (1910-88): papers incl corresp, travel journals and literary papers of Sir Thomas Herbert Parry-Williams (1887-1975), poet, essayist and scholar
Kyffin Williams (b1918), painter: corresp and papers
Pwyllgor Datblygu Addysg Gyrnraeg (Welsh Language Education Development Committee): records 1987-94
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