- Lloyd-Mostyn family, Barons Mostyn: family papers incl corresp and poetry c1776-1927 (NLW MS 24107F)
- John Bodfan Anwyl (1875-1949), Welsh scholar and Congregational minister: letters to Rev Griffith Thomas Roberts and others 1930-1938 (NLW ex 2986)
- John E Barnie (b1941), poet, writer and former editor of "Planet" magazine: personal and literary papers incl corresp with various Welsh and non-Welsh poets and literary figures
- David Daniel Bartlett (1900-1977), Bishop of St Asaph: additional papers 1950-1971
- Ray Davies (b1930), councillor and political activist: papers rel to his personal and political lives c1960-2014 (RAYDAV)
- Menna Elfyn (b1952), Welsh poet, playwright, columnist, and editor: papers incl notes, corresp, translations, scripts, reviews and incl corresp from her period in prison c1968-2017 (MENFYN)
- Walter Idris Elwyn-Jones (1900-1971), Welsh chemist and international rugby union player: papers incl diaries, corresp and photographs 1924-1971 (ELWYNES)
- Robert Geraint Gruffydd (1928-2015), Welsh scholar and critic: papers incl research notes, copies of essays, corresp rel to his role as Director of the Centre for Celtic Studies and letters and poems from Eurys Rolant
- James Hanley (1901-1985), novelist and playwright: letters (30) to author Lawrence Millman 1977-1984
- David Harries (1933-2003), Welsh musician and composer: music MSS and reel-to-reel recordings 1952-1995
- Peter Henley (fl 1967-2017), photographer: photographs, contact prints and negatives of people and places in Aberystwyth c1967-1979
- Thomas John "Jack" Howells (1913-1990), Welsh film-maker: papers rel to his film work incl corresp, scripts and working documents 1946-1989 (JACHOW)
- Thomas Terry James (1933-2016), Welsh composer and orchestral conductor: papers incl images, columns and printed material c1983-2016
- Nigel Jenkins (1949-2014), Anglo-Welsh poet, editor, journalist, psychogeographer, broadcaster, writer and lecturer: papers inc poetry, prose, plays, lectures, talks, corresp and research material
- Eluned Bebb Jones (1925-2010), radio script writer: scripts for the BBC radio programme "Natur o'n cwmpas" (Nature around us) 1955-1965 (NLW ex 2994)
- Rhydderch Thomas Jones (1935-1987), writer: film scripts written by Rhydderach Jones 1974-1987
- Shirley Jones (b1934), printmaker and publisher: corresp and ephemera rel to "Red Hen Press" 1983-2003
- Henry Watkin Lewis (1839-1897), engineer: diaries and photographs
- Helen Kaye Little (b1944), radiologist: papers rel to anti-windfarm protests at Cefn Croes and across Wales 1984-2016 (CCAG)
- David Lloyd-Howells (1942-2015), poet and composer: papers (david-lloyd-howells-papers)
- Ronald Mathias Lockley (1903-2000), author and naturalist: diaries (12) 1921-1948
- John Metcalf (b1946), composer: papers incl composition scores and material rel to Banff Centre, Alberta, Canada c1946-2017
- Alan Bertram Morgan (1897-1924), 2nd Lieutenant, 29th Squadron Royal Flying Corps: papers incl letters, diary and paybook 1917-1924 (NLW ex 2988)
- Christopher John Morgan (1944-2014), Welsh author: personal and family papers incl poems, articles, letters, notes and articles 1950-2014 (CHRGAN)
- Nina N Niedergang (fl 1980-2017), educationalist and author: research material rel to her book "Wales China - 250 years of history" 1980-2015 (ENGANG)
- Dyddgu Owen (1906-1992), writer of children's books: file containing notes and drafts of literary works 1960-1980
- Harri Elwyn Pritchard Jones (1933-2015), Welsh language author, critic, and psychiatrist: papers
- William Rees (c1824-1898), Welsh clergyman: commonplace book with MS and printed notes c1880-1898 (NLW MS 24115)
- Edward "Ted" Richards (1893-1973), Welsh musician: papers incl material rel to wife, Gwenfron M Barrett and niece, Nansi Richards c1929-1971
- Howard Lloyd Roberts (1879-1935), Lance Corporal and illustrator: trench diary 1916
- Berta Ruck (1878-1978), novelist: holograph poem entitled "Birds in Winter" and watercolour illustration (NLW MS 24044D (amryw))
- Nansi Selwood (b1921), Welsh author and bard: papers incl manuscripts and corresp
- Ernest Lewis Thomas (1904-1983), Welsh author: scrapbooks incl reviews of his published works 1950-1961 (NLW ex 2982)
- Angharad Tomos (b1958), author: typescript with corrections of "Once Upon a dawn" (English translation of "Wele'n gwawrio") c2004 (ATOMOS)
- Moira Morven Vincentelli (fl 1971-2018), artist, lecturer, curator and writer: papers incl corresp, research notes and slides rel to exhibitions she has curated c1972-1993 (VINCENT)
- Arthur William Wrigley (1907-1980), author: manuscripts of "Reminiscences of Arthur W Wrigley" and "A Short history of the Toller Chapel Sunday School, 1883-1891" c1883-1910 (NLW MS 24109)
- Unnamed male (fl 1822), Welsh travel diarist: travel journal of a tour through parts of Monmouthshire, Glamorgan and Breconshire with Rev Barton and Mrs Mary Bouchier incl handwritten religious notes 1822 (NLW ex 2962)
- Unnamed travel diarist (fl 1916-1918): diary of several cycling holidays in England and Wales incl photographs and drawings 1916-1918 (NLW MS 24113)
- Llanvihangel Rail Way: papers incl letters and minutes 1810-1823 (NLW ex 2978)
- RH Williams Associates, architects, Caernarfon: records
- Cymdeithas yr Iaith Gymraeg (Welsh Language Society): Glamorgan-Gwent area: corresp rel to the use of the Welsh language in shops and businesses 1990-2000
- Ebenezer Presbyterian Church, Cwmrhydyceirw, Morriston: records incl accounts, minutes, corresp and related papers 1940-2004 (EBECWM)
- Forward Movement Church, St Thomas, Swansea: records incl registers, accounts, minutes, corresp c1898-2001 (PORTNT)
- Island Farm Prisoner of War Camp, Bridgend: papers incl nominal rolls, corresp, photographs and other biographical accounts collected by Capt Ted Lees, Intelligence Officer and Interpreter 1945-1985 (NLW MS 24094)
- Llanelly Trades Council and Divisional Labour Party: minute books 1932-1940 (DEIKIN)
- North Wales Women's Liberal Federation: records incl minutes and papers 1929-1985 (NWLIBW)
- Parc Womens Institute: papers incl corresp rel to the Welsh language 1965-1978 (NLW ex2995)
- Plaid Cymru: records incl National Council papers c1925-1994 (PLAMRU)
- Religious Education Movement Wales (REMW): papers 2004-2016
- Sandfields Presbyterian Church, Port Talbot: records incl accounts, minutes and members register 1949-2016
- St David's School, independent girls school, Ashford: papers incl minutes, accounts, corresp, applicants' books, attendance books, wages books c1567-1974 (WELOOL)
- Trinity Chapel, Clydach: records incl corresp, accounts and minutes c1916-2002 (CAPCLY)
- Wales Deaf Broadcasting Council: papers incl minutes, corresp, and Treasurer's papers 1987-2016
- Welsh Development Agency: papers, printed material and photographs rel to Bet Davies, Director of Media and Communication for the WDA 1986-2012
- John Glyn Davies (1870-1953), poet, Professor in Welsh: papers incl letters, family papers (JGILES)
- Meredydd Evans (1919-2015), musicologist, performer, language campaigner: additional corresp 1956-2015 (Archif Meredydd Evans a Phyllis Kinney)
- David Lloyd George (1863-1945), 1st Earl Lloyd George of Dwyfor, statesman: handwritten letter to Frederick William Hughes rel to Welsh farmers aiding the war effort 1917 (NLW MS 24045F (amryw))
- Sean Hales (1880-1922), Irish political activist: holograph letter and transcript describing his life while incarcerated at Frongoch camp 1916 (NLW MS 24044D)
- Robert Williams Parry (1884-1956), poet: letter (1) with poems (englymion) in his hand 1891 (NLW MS 24044D (amryw))
- Accounts for land revenues in counties of Pembroke, Carmarthen, Cardigan, Brecon, Radnor, Glamorgan and Monmouth to Sir Henry Fox, Lord Holland and Richard Bateman, Receivers General of the King's Revenues in South Wales 1736-1758 (NLW Deeds 1955-1961)
- Bodelwyddan family: pedigree roll created by Griffith Hughes 1660 (NLW MS 24108G)
- Dugdale family of Llwyn: additional Montgomeryshire (Llwyn) estate and family papers c1851-1952 (LLWYN)
- List of grievances about finances in the Welsh Marches presented by Francis Bacon to James VI & I 1610 (NLW MS 24045F (amryw))
- Pedigree of John Bowen, from Bleddyn app Maenarch and earlier derived from a lost roll of 1608 by Thomas Jones of Fountain Gate, Tregaron 1819 (NLW MS 24111G)
- Pedigree of Gawen Goodman of Ruthin, first drawn and set down by Simwnt Fychan and newly drawn by Richarde Thomlyns of Denbigh 1584
- Pedigree roll showing the descent of the Watkins family, from Bennet Penclawdd to William and Thomas Watkins of Usk, possibly compiled by Walter Hopkins or one of his assistants c1637 (NLW MS 24114G)
- Dolobran panel depicting the arms of the Lloyd family impaling Stanley with numerous quarterings and impalement 1650 (NLW MS 24110)
- Trayan manor, Denbighshire: rent roll 1723-1724
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National Library of Wales: Department of Collection Services
